I'm not sure where this performance was, but Prima & Smith's version of "That Old Black Magic" is one of their best-loved tunes.
Keely and Louie appeared in the Robert Mitchum 1958 classic Thunder Road. In this clip, Mitchum doesn't appreciate the loudmouth drunk whose obnoxious laughing nearly drowns out Keely's performance of "Won't You Come Home Bill Bailey."
In the mid '60s she released Keely Smith Sings the John Lennon—Paul McCartney Songbook, a collection of Beatles tunes. Here's a swingin' version of "Please Please Me."
But this was her first solo hit, from 1957. Keely, wherever you are, we wish you love.